Archiv Vorträge

Raum: Seminar rooms 1-2 Ort: MPI CPfS
Abstract: Superconducting qubits equipped with quantum non-demolishing readout and active feedback can be used as information engines to probe and manipulate microscopic degrees of freedom, whether intentionally designed or naturally occurring in their environment. In the case of spin systems, the required magnetic field bias presents a significant challenge for superconductors and Josephson junctions. Using a nano-Josephson junction, of only 20 nm cross-section, and superconducting granular Aluminum films with critical field above 5 Tesla, we operate a flux qubit in magnetic field of up-to 1.2 Tesla. Remarkably, the spectrum and coherence of the qubit remain stable in this entire range, and we can observe the freezing of a paramagnetic spin ensemble coupled to the qubit. [mehr]
Abstract: Chemistry is all about understanding and controlling the properties of matter -- Where are the electrons? How do particular arrangements of atoms and bonds result in the zoo of behaviors known in matter? What new properties can be created by arranging atoms in unnatural configurations? Today, there are about 50 million known chemical compounds. Where and how will the next billion be discovered, and what new properties will they have [1]? In this talk, I will highlight the progress being made to address these questions, with a particular emphasis on the confluence of quantum materials, quantum information science, and data science. Examples will include our forays into closed loop coupling of human experiment and AI/ML prediction for superconductor discovery [2,3], the creation of approaches for the systematic design of complex materials [4], and the importance of advancing old and new materials synthesis methods [5,6]. As time permits, I will highlight how these methods come together to enable discovery of new chemistry, and new physics, and provide my perspective on the future of materials design, synthesis, and discovery. 1. https://dx.doi.org/10.1021/acs.accounts.8b00382 2. https://doi.org/10.1038/s41524-023-01131-3 3. https://openreview.net/forum?id=SfEsK3O2KT 4. https://doi.org/10.1021/jacs.4c08941 5. https://doi.org/10.1021/acs.chemmater.3c03077 6. https://doi.org/10.1038/s41535-022-00527-6 [mehr]

Self-assembly models for crystal growth and phase transitions

How can we make new materials and better understand how their underlying structures form? The direct observation of crystal growth and transitions remains supremely challenging, but gaining insight into these fundamental processes is central to our quest of creating materials in a rational and targeted way, connecting structure to functionality. We build self-assembly models, study how they react to perturbations on the particle and system levels, and investigate their impact on crystal growth and transformation pathways. We use simple coarse-grained models to gain systematic insights into the phenomena that lead to the crystallization of complex crystal structures, partial disorder, or magic-size assemblies, allowing us to derive the essential principles that govern the formation of materials' structures. Our goal is to use these insights to find ways to tailor crystallization pathways and to create new functional materials. Our work promises to establish new pathways to materials design through simulations, which explicitly incorporate and explore phase transformation kinetics. [mehr]
Abstract: We investigate the lattice relaxation effect on moir´e band structures in twisted bilayer MoTe2 with two approaches: (a) large-scale plane-wave basis first principle calculation down to 2.88 deg, (b) transfer learning structure relaxation + local-basis first principles calculation down to 1.1 deg. Two types of van der Waals corrections have been examined: the D2 method of Grimme and the density-dependent energy correction. We note the density-dependent energy correction yields a continuous evolution of bandwidth with twist angles. Including second harmonic of intralayer potential/interlayer tunneling and the strain induced gauge field, we develop a more complete continuum model with a single set of parameters for a wide range of twist angles, and perform many-body simulations at v=-1,-2/3, -1/3. We further identify a series of C=1 Chern bands around 2 from Wilson loop and edges state calculation, which serves as the foundation point for even-denominator non-Abelian states. [mehr]
Abstract: Non-collinear chiral antiferromagnet (AFM) Mn3Sn is an attractive material since this AFM exhibits a Néel temperature of 420 K and a non-negligible magneto-optical Kerr effect (MOKE) due to magnetic-octupole order and topological Weyl nature. Despite extensive research on ultrafast magnetization dynamics in ferromagnets and ferrimagnets, investigations into such chiral AFMs are still in their very early stages. In particular, magnetic damping significantly influences both the energy efficiency and operational speed of the device aiming to utilize the electronic spin degree of freedom, thus further understanding is demanded. Here we investigate, for the first time, time-resolved magneto-optical Kerr effect for Mn3Sn films with a perpendicular magnetic anisotropy to gain insight into the physics of octupole dynamics. The films were prepared using magnetron sputtering technique. The film stacking structure is single crystalline MgO (110) sub./W(2) /Ta(3) /Mn3Sn(30) /MgO(1.3) /Ru(1) (thickness is in nm). The time-resolved MOKE (TR-MOKE) was measured using an all-optical pump-probe technique. The out-of-plane magnetic-octupole dynamics is induced by the pump laser pulse and is detected via MOKE for a probe laser pulse. We observed an ultrafast change of Kerr rotation angle at the zero delay, which is attributed to ultrafast collapse of magnetic octupole order. We also observed the damped-oscillation which would be attributed to GHz-frequency magnetic octupole order dynamics. [mehr]
Abstract: Ni-Mn based Heusler alloys undergo a first-order magneto-structural transition (FOMST) from high-temperature high magnetic austenite to low-temperature low magnetic martensite. The FOMST can be induced by external stimuli such as magnetic fields, uniaxial stress, or temperature. The sensitivity of FOMST to external stimuli results in large caloric effects and can be used for multicaloric solid-state cooling. A disadvantage of Ni-Mn-based Heusler alloys is their brittleness, limiting the shaping of those alloys required for further application. We used microstructure design by suction casting or additive manufacturing (AM) to process alloys with beneficiary microstructure to increase mechanical stability and cyclic performance. In addition, AM also enables the processing of complex geometries. We also investigate the correlation of microstructure and the thermal hysteresis of the FOMST and the transition width. By in-situ microscopy, we can identify the nucleation sides of the FOMST and the defect acting as pinning sides for the propagation of the phase transition. The FOMST and thermal hysteresis can be specifically designed for multicaloric cooling cycles by tailoring the processing method, parameters, and particle size. In addition, microstructural design by DED, PBF-LB, SPS, or hot compaction can significantly improve the mechanical and cyclic stability of brittle Heusler alloys. This work is supported by ERC (Adv. Grant "Cool Innov") and DFG 527201505 and CRC/TRR 270 "HoMMage". [1] F. Scheibel et al., Energy Techn. 6, 1397 (2018), DOI :10.1002/ente.201800264 [2] L. Pfeuffer et al., Acta Mater. 221, 117390 (2021), DOI:10.1016/j.actamat.2021.117390 [3] F. Scheibel et al., Materialia 29, 101783 (2023), DOI:10.1016/j.mtla.2023.101783 [4] F. Scheibel et al., Adv. Eng. Mater. 24, 2200069 (2022), DOI:10.1002/adem.202200069 [mehr]
Frontiers of topological quantum matter: linked Weyl rings and ideal Weyl ferromagnets Quantum science is driven by the synthesis of state-of-the-art quantum materials and the characterization of their exotic topological states [1-7]. In the first part of this talk, I introduce our discovery of linked Weyl rings in the room temperature Heusler ferromagnet Co2MnGa using high-resolution soft X-ray ARPES [1,2]. By combining ideas in condensed matter physics and knot theory, I explicitly draw the Weyl link diagram for the quantum state and show a linking number of (2,2,2), providing a direct experimental measurement of a new kind of topological invariant in physics. In the second part of this talk, I introduce our observation of a semimetallic Weyl ferromagnet in thin films of (Cr,Bi)2Te3 [3]. In transport, we find a record bulk anomalous Hall angle > 0.5 along with non-metallic conductivity, a regime sharply distinct from established Weyl materials and conventional ferromagnets. Together with density functional theory (DFT), our data suggest a semimetallic Fermi surface composed of two Weyl points, with a giant separation > 75% of the linear dimension of the bulk Brillouin zone, and no other electronic states. Using non-equilibrium molecular beam epitaxy (MBE), we widely tune the electronic structure, allowing us to annihilate the Weyl state and visualize a Murakami-type topological phase diagram with broad Chern insulating, Weyl semimetallic and magnetic semiconducting regions. Our discovery of a topological quantum link and semimetallic Weyl ferromagnet suggests new approaches to non-Abelian quantum states, as well as materials synthesis methods relevant to quantum technology. 1. I.B. et al. Nature 604, 647 (2022) 2. I.B. et al. Science 365, 6459 (2019) 3. I.B. et al. Nature, under review 4. Max T. Birch, I.B. et al. Nature, in press (2024) 5. M. Z. Hasan, G. Chang, I.B. et al. Nat. Rev. Mat. 6, 784 (2021) 6. D. Sanchez*, I.B.* et al. Nature 567, 500 (2019) 7. S. Xu*, I.B.* et al. Science 349, 613 (2015) [mehr]

Local Thermodynamic Measurements of Semiconductor Moiré Systems

Wichtige Hinweise zur COVID-19-Pandemie: Bitte haben Sie Verständnis, dass wir nach Ihrer Registrierung nochmals mit Ihnen in Kontakt treten. Um alle beteiligten Personen ausreichend zu schützen, möchten wir sichergehen, dass die geltenden Regeln rund um die COVID-19-Pandemie zu jeder Zeit eingehalten werden. [mehr]

Comprehensive Course on Topological Systems: Band structure calculations - tight binding

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all are involved in our world-leading research activities in this field. The series of lectures is particularly targeted at PhD students and other junior researchers. As several scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a great overview over the research activities at our institute in this field. [mehr]

Comprehensive Course on Topological Systems: Calculation of topological invariant-I

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all are involved in our world-leading research activities in this field. The series of lectures is particularly targeted at PhD students and other junior researchers. As several scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a great overview over the research activities at our institute in this field. [mehr]

Comprehensive Course on Topological Systems: Applications of topological materials/Catalysis

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all are involved in our world-leading research activities in this field. The series of lectures is particularly targeted at PhD students and other junior researchers. As several scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a great overview over the research activities at our institute in this field. [mehr]

Comprehensive Course on Topological Systems: Table-top experiments for high energy physics

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all are involved in our world-leading research activities in this field. The series of lectures is particularly targeted at PhD students and other junior researchers. As several scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a great overview over the research activities at our institute in this field. [mehr]

Comprehensive Course on Topological Systems: Materials and Topology

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all are involved in our world-leading research activities in this field. The series of lectures is particularly targeted at PhD students and other junior researchers. As several scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a great overview over the research activities at our institute in this field. [mehr]

Comprehensive Course on Topological Systems - Magnetic topological materials

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all are involved in our world-leading research activities in this field. The series of lectures is particularly targeted at PhD students and other junior researchers. As several scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a great overview over the research activities at our institute in this field. [mehr]

Comprehensive Course on Topological Systems - Electron Transport

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all are involved in our world-leading research activities in this field. The series of lectures is particularly targeted at PhD students and other junior researchers. As several scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a great overview over the research activities at our institute in this field. [mehr]

Comprehensive Course on Topological Systems - Transport Experiments

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all areinvolved in our world-leading research activities in this field.The series of lectures is particularly targeted at PhD students and other junior researchers. Asseveral scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a greatoverview over the research activities at our institute in this field. [mehr]

Comprehensive Course on Topological Systems - Electron Transport I

Comprehensive Course on Topological Systems
The course on topological systems is offered by several researchers at MPI CPfS who all areinvolved in our world-leading research activities in this field.The series of lectures is particularly targeted at PhD students and other junior researchers. Asseveral scientists will give lectures on their respective research area, the course will offer abroad introduction into the field of topological materials and at the same time provide a greatoverview over the research activities at our institute in this field. [mehr]
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